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Monolithic Integration of High-Temperature
Superconductor
with Ferroelectric and Ferrite for Microwave
Devices
Quanxi Jia
Superconductivity Technology Center
Los Alamos National Laboratory
Los Alamos, NM 87545
Since the discovery of high-temperature superconducting (HTS)
materials, electrically tunable and active microwave device applications of
these materials have been explored both experimentally and theoretically.
Passive microwave elements incorporating HTS films have started to find
application in high quality filters, resonators, delay lines, etc., operating at
or around the liquid nitrogen temperature. Another emerging area where the HTS
materials play a big role is in tunable microwave electronics. It is desirable
for many microwave applications to tune the device characteristics. The
fundamental aspect of a tunable microwave device is based on the change of the
microwave propagation factor by physical, electrical, or magnetic means. For
example, electric tuning employs the nonlinearity of ferroelectric materials
under DC bias, whereas magnetic tuning utilizes the nonlinear magnetization of
the ferrite under a magnetic field. When an electromagnetic wave travels in a
medium of dielectric constant e and magnetic
susceptibility m, its phase speed is vp
= (em)-1/2
and its intrinsic impedance is Z = (m/e)1/2.
When the media include a nonlinear dielectric, such as SrTiO3 (STO),
applying an electric field will change its e.
Similarly, when a ferrimagnetic material, such as ferrite, Y3Fe5O12 (YIG), is incorporated in the media, applying a magnetic field will change its m.
The frequency and phase characteristics of the microwave device can thus be
tuned. The drawback of these devices operated at room temperature, however, is
their higher signal losses from the patterned metal circuits (typically Cu).
Microwave propagation can be dramatically improved if superconductors can be
used to replace the normal conductors. From a materials point of view, the
successful demonstration of high performance active microwave devices relies on
the full integration of high quality tunable media with the superconductors. In
other words, the ultimate goal of monolithic integration of superconductors with
tunable media is to combine dissimilar materials with complementary
functionalities on a single platform and to have optimum performance from each
layer.
YBCO/SrTiO3 on a single crystal substrate for electrically tunable
devices
Ideal performance of functional materials is best achieved by
minimizing crystallographic imperfections such as grain boundaries, and chemical
imperfections such as variations in the stoichiometry. To this end, single
crystal substrates are often used as the starting templates. For example,
excellent structural and chemical compatibilities make it possible to grow high
quality STO on LaAlO3 or MgO substrates. YBCO can be epitaxially
grown on STO thereafter. Figure 1 shows the microwave reflection S11
and transmission S21 vs frequency at 4 K under varying
bias voltages (average values applied at each pole) for a 3-pole half-wave
bandpass coplanar waveguide (CPW) filter incorporating a 1.2 mm-thick
STO layer and a 0.4 mm-thick YBCO electrode layer on
a LaAlO3 substrate, where the gap between the centerline and the
ground-plane is 30 mm [1]. If the broadband tuning of
the filter is not required, one would be better off using much thinner STO
films, still allowing fine tuning of the filter profile. The use of thinner STO
films as well as large dc biases should reduce dielectric losses significantly.
Also, the required bias voltages can be reduced by designing circuits with
smaller centerline-to-ground plane gaps.

YBCO on polycrystalline YIG for magnetically tunable devices
Ferrite components have traditionally played important roles
in microwave systems. Their inherent capability to meet high power-handling
requirements with high efficiency has made them the preferred technology for
numerous radar applications. It has been demonstrated that the optimum coupling
of rf signal in the superconductor to the ferrite occurs where a monolithic
structure is used in which the superconductor is deposited directly on the
ferrite substrate [2]. This configuration also simplifies device design and
packaging.
The deposition of high quality YBCO on polycrystalline
YIG represents an advance of great technical significance. Ceramic substrates
are not only readily available in sizes needed for devices, but they are
dramatically less expensive than single-crystal substrates that for many
chemical compositions may not even be attainable by known processing methods.
However, the deposition of device quality YBCO on a polycrystalline YIG
substrate can be a formidable challenge because of the inherent crystallographic
incompatibility of the two materials and the lack of an epitaxial template for
the growth of well-oriented YBCO. Recently, it has been demonstrated that highly
oriented YBCO films can be grown on a biaxially textured YSZ layer that is
deposited by an ion-beam-assisted-deposition (IBAD) process [3]. Figure 2
schematically shows the filter fabricated from YBCO on polycrystalline ferrite
YIG with an IBAD-YSZ template as described in [3]. The tunability is what has
been expected from the YIG, and the excess loss is believed to be from the
ferrite [4].

YBCO/SrTiO3 on polycrystalline YIG for
dual-tuning devices
Ferrite and ferroelectric materials individually provide the
magnetic and the electrical tunability for adaptive microwave devices,
respectively. The adaptability will increase significantly if a microwave device
can be simultaneously tuned by both magnetic and electrical techniques. In the
tunable filter case, for example, the dual-tuning allows not only for fine
tuning of the filter profile to achieve symmetric and optimum filter
characteristics electrically but also for broadband magnetic tuning of the
filter passband to demonstrate adaptive filter response over a wide frequency
range.
Figure 3 shows a cross-sectional view of the architecture
used for integration among polycrystalline YIG, STO, and YBCO. Using a template
of biaxially oriented MgO, deposited by an IBAD technique, device quality STO
and YBCO films on polycrystalline YIG substrates have demonstrated [5]. The
effort to fabricate high performance devices based on this monolithic integrated
system is underway.

References
[1] A. T. Findikoglu, Q. X. Jia, X. D. Wu, G. J. Chen, T.
Venkatesan, and D. W. Reagor, Appl. Phys. Lett. 68, 1651 (1996).
[2] D. E. Oates and G. F. Dionne, IEEE Trans. Appl. Supercond.
9, 4170 (1999).
[3] Q. X. Jia, A. T. Findikoglu, P. Arendt, S. R. Foltyn, J.
M. Roper, J. R. Groves, J. Y. Coulter, Y. Q. Li, and G. F. Dionne, Appl. Phys.
Lett. 72, 1763 (1998).
[4] D. E. Oates, A. C. Anderson, and G. F. Dionne, Mat. Res.
Soc. Symp. Proc. 603, 113 (2000).
[5] Q. X. Jia, J. R. Groves, P. N. Arendt, P. Lu, and F. Miranda, Integrated
Ferroelectrics 42, 71 (2002).
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